The term 'VILLAIN's Look' can be summarized by two crossword solutions: SNEER and LEER. A SNEER is a facial expression of contempt or scorn, usually characterized by a curled lip and a scornful look. A LEER is a facial expression of someone looking at someone else with a suggestive or lascivious look. Both expressions are often associated with villains in literature and film, as they are used to convey a sense of malicious intent.