The term 'Tangle of Hair' can be described by two crossword solutions: MAT (3 letters) and SNARL (5 letters). MAT is a type of coarse fabric made from jute, hemp, or other vegetable fibers. It is often used to make mats, rugs, and other floor coverings. SNARL is an expression of anger or frustration, usually accompanied by a facial expression of displeasure. It can also refer to a tangled mess of hair. Therefore, the term 'Tangle of Hair' can be described as a coarse fabric-like mess of hair that expresses anger or frustration.