The term 'Pick of the Bunch' is a phrase used to describe something that is the best or most desirable of a group. The two crossword solutions for this phrase are 'ELITE' (5 letters) and 'CHOICE' (6 letters). ELITE is defined as being of the highest quality or having the most desirable characteristics, while CHOICE implies that the item is the best or most desirable of a group. Both words can be used to describe something that is the pick of the bunch.