The term '007 Portrayer' refers to the actors who have played the iconic James Bond character in the long-running film series. The six solutions to the crossword are Timothy Dalton (6 letters), Roger Moore (5 letters), Sean CONNERY (7 letters), Roger Moore (10 letters), Daniel Craig (11 letters), and Pierce Brosnan (13 letters). Timothy Dalton was the third actor to portray James Bond, appearing in two films in the late 1980s. Roger Moore was the fourth actor to play the role, appearing in seven films between 1973 and 1985. Sean CONNERY was the first actor to portray James Bond, appearing in seven films between 1962 and 1983. Roger Moore was the longest-serving actor in the role, appearing in seven films between 1973 and 1985. Daniel Craig is the sixth actor to portray James Bond, appearing in four films since 2006. Finally, Pierce Brosnan was the fifth actor to portray James Bond, appearing in four films between 1995 and 2002.